Abstract
Electrons floating on condensed noble-gas substrates form a remarkably clean material system that is minimally influenced by the underlying host material, and recent experiments have explored their potential as a qubit platform. In particular, single electrons floating on solid neon thin films have attracted significant interest because they exhibit long coherence times when probed with superconducting circuits at frequencies around 6 GHz. Surprisingly, however, the energy spectrum of these qubits resembles that of a two-level-system defect more than the spectrum expected from the Coulomb potential defined by the bias electrodes. In this thesis, I first review floating-electron systems and the experimental methods used to probe their quantum states. I then show that electron-on-neon qubits with transition frequencies of a few GHz are observed only on neon films deposited on silicon surfaces, and not on neon films deposited on sapphire. Motivated by this observation, I propose a model in which a floating electron on the neon surface interacts with fixed positive charge defects in the native oxide at the silicon surface. Using realistic parameters, this model reproduces the observed voltage-dependent transition frequency and coupling strength of electron-on-neon qubits.
Committee Chair
Kater Murch
Committee Members
Dafei Jin; Erik Henriksen; Li Yang; Sheng Ran
Degree
Doctor of Philosophy (PhD)
Author's Department
Physics
Document Type
Dissertation
Date of Award
7-28-2026
Language
English (en)
DOI
https://doi.org/10.7936/1wqw-we75
Recommended Citation
Zheng, Kaiwen, "On the Origin of Coherent Gigahertz Two-Level States in Electron-on-Neon Systems" (2026). Arts & Sciences Graduate Student Theses and Dissertations. 3849.
The definitive version is available at https://doi.org/10.7936/1wqw-we75